由于狗狗的体重为20斤,夺调侃所以补液的葡萄糖量也是与体重有关的。
除此之外,态耐采用温和的电化学还原法,在室温下即可完成催化剂的制备,显著降低的反应温度可以有效防止金属原子团聚。第一作者:克被陈雅文 通讯作者:克被李佳,刘建国 通讯单位:南京大学/华北电力大学 论文DOI:10.1016/j.apcatb.2021.120830 全文速览绿色氢能的发展必须要使用大量的贵金属Pt作为电催化剂来加速氢析出(HER)反应的发生,然而高昂的价格使得研究人员必须寻找降低成本的方法。
(d)PtNP/NCCo1NC、夺调侃Pt1/Co1NC、PtNP/NC和商业20wt%Pt/C的HER催化活性在室温下使用三电极系统进行测量。所得PtNP/NC中的铂的质量分数为0.5wt%,态耐而在Pt1/Co1NC中为0.4wt%,同时,Co在Pt1/Co1NC中为0.17wt%。作为对照样品,克被PtNP/NC的制备方法与Pt1/Co1NC类似。
其质量活性可达32.4Amg-1Pt,夺调侃20mV处的TOF为32.86s-1。以第一作者身份已发表的论文:1.RuiDing,RanWang,YiqinDing,WenjuanYin,YideLiu,JiaLi*,JianguoLiu*,DesigningAI-aidedanalysisandpredictionmodelsfornonpreciousmetalelectrocatalyst-basedprotonexchangemembranefuelcells,AngewandteChemieInternationalEdition,2020,59,19175-19183.2.RuiDing,YawenChen,XiaokeLi,ZhiyanRui,KangHua,YongkangWu,XiaoDuan,XuebinWang,JiaLi*,andJianguoLiu*, AtomicallyDispersed,Low-CoordinateCo–NSitesonCarbonNanotubesasInexpensiveandEfficientElectrocatalystsforHydrogenEvolutionSmall,2021,DOI:10.1002/smll.202105335,Accepted3.RuiDing;YawenChen;PingChen;RanWang;JiankangWang;YiqinDing;WenjuanYin;YideLiu;JiaLi;JianguoLiu,ACSCatalysis,2021,11,97984.RuiDing,YiqinDing,HongyuZhang,WenjuanYin,RanWang,ZihanXu,YideLiu,JiankangWang,JiaLi*,JianguoLiu*,Applyingmachinelearningtoboostthedevelopmentofhigh-performancemembraneelectrodeassemblyforprotonexchangemembranefuelcells,JournalofMaterialsChemistryA,2021,9,6841.(insidecover)5.RuiDing,YideLiu,ZhiyanRui,JiaLi*,JianguoLiu*,ZhigangZou,FacileGraftingstrategysynthesisofsingle-atomelectrocatalystwithenhancedORRperformance,NanoResearch,2020,13,1519-1526.(backcover)6.RuiDing#,WenjuanYin#,GangCheng,YawenChen,JiankangWang,RanWang,ZhiyanRui,JiaLi,JianguoLiu,EnergyandAI,2021,5,100098.李佳(通讯作者)2020年8月至今,态耐特任副研究员,态耐南京大学2017年11月-2020年7月,博士后,南京大学2012年9月-2017年9月,博士研究生,大连理工大学2008年9月-2011年7月,硕士研究生,内蒙古大学2004年9月-2008年7月,本科,内蒙古大学研究方向:燃料电池低铂及非贵金属电催化剂代表性论文:[1]RuiDing#,WenjuanYin#,GangCheng,YawenChen,JiankangWang,RanWang,ZhiyanRui,JiaLi,JianguoLiu,EnergyandAI,2021,5,100098.[2]RuiDing,YawenChen,XiaokeLi,ZhiyanRui,KangHua,YongkangWu,XiaoDuan,XuebinWang,JiaLi*,andJianguoLiu*, AtomicallyDispersed,Low-CoordinateCo–NSitesonCarbonNanotubesasInexpensiveandEfficientElectrocatalystsforHydrogenEvolutionSmall,2021,DOI:10.1002/smll.202105335,Accepted[3]RuiDing,YawenChen,XiaokeLi,ZhiyanRui,KangHua,YongkangWu,XiaoDuan,XuebinWang,JiaLi*,andJianguoLiu*, AtomicallyDispersed,Low-CoordinateCo–NSitesonCarbonNanotubesasInexpensiveandEfficientElectrocatalystsforHydrogenEvolutionSmall,2021,DOI:10.1002/smll.202105335,Accepted[4]YawenChen,RuiDing,JiaLi*,JianguoLiu*,Highlyactiveatomicallydispersedplatinum-basedelectrocatalystforhydrogenevolutionreactionachievedbydefectanchoringstrategy,AppliedCatalystB:Environmental,2022,301,120830[5]RuiDing;YawenChen;PingChen;RanWang;JiankangWang;YiqinDing;WenjuanYin;YideLiu;JiaLi;JianguoLiu,ACSCatalysis,2021,11,9798[6]RuiDing,YiqinDing,HongyuZhang,WenjuanYin,RanWang,ZihanXu,YideLiu,JiankangWang,JiaLi*,JianguoLiu*,Applyingmachinelearningtoboostthedevelopmentofhigh-performancemembraneelectrodeassemblyforprotonexchangemembranefuelcells,JournalofMaterialsChemistryA,2021,9,6841.(insidecover)[7]RuiDing,RanWang,YiqinDing,WenjuanYin,YideLiu,JiaLi*,JianguoLiu*,DesigningAI-aidedanalysisandpredictionmodelsfornonpreciousmetalelectrocatalyst-basedprotonexchangemembranefuelcells,AngewandteChemieInternationalEdition,2020,59,19175-19183.[8]RuiDing,YideLiu,ZhiyanRui,JiaLi*,JianguoLiu*,ZhigangZou,FacileGraftingstrategysynthesisofsingle-atomelectrocatalystwithenhancedORRperformance,NanoResearch,2020,13,1519-1526.(backcover)[9]JiaLi,XiangZhu,JianyuWang,ZhiyanRui,ShiqiaoZhang,YuxinLi,RuiDing,WenxiangHe,JianguoLiu*,ZhigangZou,Iron-containingporphyrinsself-assembledonZnOnanoparticlesaselectrocatalyticmaterialsforoxygenreduction,ACSAppliedNanoMaterials,2020,3,742-751.[10]JiaLi,Jin-XunLiu,XueqiangGao,BryanR.Goldsmith,YuanyuanCong,ZihuiZhai,ShuMiao,QikeJiang,YongDou,JunhuWang,QuanShi,XinwenGuo,DonghaiWang,HongmeiYu,Wei-XueLi*,YujiangSong*,Nitrogen-dopedgraphenelayersforelectrochemicaloxygenreductionreactionboostedbylatticestrain,JournalofCatalysis,2019,378,113-120.[11]JiaLi,YujiangSong*,GaixiaZhang,HuiyuanLiu,YirenWang,ShuhuiSun*,XinwenGuo,Pyrolysisofself-assembledironporphyrinoncarbonblackascore/shellstructuredelectrocatalystsforhighlyefficientoxygenreductioninbothalkalineandacidicmedium,AdvancedFunctionalMaterials,2017,27,1604356.(frontcover)[12]JiaLi,HuiyuanLiu,YangLv,XinwenGuo,YujiangSong*,Influenceofcounterelectrodematerialduringaccelerateddurabilitytestofnon-preciousmetalelectrocatalystsinacidicmedium,ChineseJournalofCatalysis,2016,37,1109-1118.[13]JiaLi,YanXie,ShushuangLi,YangzhiBai,XinwenGuo*,BaolianYi,YujiangSong*,Graphenesupportedfoam-likeplatinumelectrocatalystforoxygenreductionreaction,MaterialsResearchExpress,2014,1,025045.[14]WeifengSi‡,JiaLi‡(‡Co-firstauthors),HuanqiaoLi,ShushuangLi,JieYin,HuanXu,XinwenGuo,TaoZhang,YujiangSong*,Light-controlledsynthesisofuniformplatinumnanodendriteswithmarkedlyenhancedelectrocatalyticactivity,NanoResearch,2013,6,720-725.邮箱:[email protected]刘建国(通讯作者,课题组负责人)刘建国,华北电力大学二级教授,博士生导师,入选国家高层次人才计划。
克被[email protected]本文由刘建国课题组供稿。
众所周知,夺调侃随着AreaD/AreaG比率的增加,相应碳材料的无序度增加,表明材料体系有更多的缺陷。态耐本工作通过发展一种基于支撑管中管夹层形态的更硬的空心管设计来解决大变形恢复能力和低比阻尼问题。
它还正确地预测,克被较厚的Ni层(较大的外管直径)和碳质量向外管的重新分配将导致较高的转动惯量,因此弯曲模量较高。相反,夺调侃低长径比试样表现出应变硬化,这种硬化随着约束程度的增加而更加明显。
图4. 具有不同样品纵横比和结构的原位SEM压缩测试图5.最佳阻尼系数(E0.5η/ρ)与比模量(E/ρ)五、态耐结论与展望。克被本工作希望该研究结果能够启发基于局部结构元素优化的低密度材料新的先进结构设计的发展。
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